Akainu would be my first guess. Arlong too. A lot of main antagonist mainly (Enel, Kuro, Crocodile, Orochi, Doffy etc.). I can only really dislike a character based on their value.
Vergo.
He got great design, caught the traitor and very competent.
I just don't like he is too overpowered, for a side villain he ran through gauntlet Kaido style, schooling pre TS Luffy's biggest rival (Smoker) and can only be beaten with hax.
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Vergo felt more threatening than 5 Egghead Gorosei.
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