Brook dying makes sense. Because if he keeps on living, he’d inevitably end up alone after all the SHs die. Brook is the oldest, he’s lived a full life, and tbh, he’s the least consequential SH.
If anyone is going to have a death it is going to be brook. My theory is that Brook’s awakening will allow him to revive one person, but at the cost of his own life.
I could see Zoro dying and brook reviving him at the cost of his own life. Zoro would effectively gain some of Brook’s powers due to dying and being revived(he wouldn’t get the yomi yomi no mi tho, just a more powerful soul due to surfing death).
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Zoro dying and being revived would also probably lead to “king of hell” replacing pirate hunter as his epithet.
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As for who would kill zoro and ultimately brook, it would probably be Imu. This would be another moment similar to hakai or thriller bark. I don’t see anyone else who would be able to do it.